Horonobe Underground Research Laboratory Project Investigation Report for the 2022 Fiscal Year

Nakayama, Masashi

JAEA-Review 2023-032, 159 Pages, 2024/02

JAEA-Review-2023-032.pdf:19.37MB

The Horonobe Underground Research Laboratory (URL) Project is being pursued by the Japan Atomic Energy Agency (JAEA) to enhance the reliability of relevant technologies for geological disposal of high-level radioactive waste through investigating the deep geological environment within the host sedimentary rocks at Horonobe Town in Hokkaido, north Japan. In the fiscal year 2022, we continued R&D on "Study on near-field system performance in geological environment", "Demonstration of repository design options", and "Understanding of buffering behaviour of sedimentary rock to natural perturbations". These are identified as key R&D on challenges to be tackled in the Horonobe underground research plan for the fiscal year 2020 onwards. Specifically, "full-scale engineered barrier system (EBS) performance experiment" and "solute transport experiment with model testing" were carried out as part of "Study on near- field system performance in geological environment". "Demonstration of engineering feasibility of repository technology" and "evaluation of EBS behaviour over 100C" were addressed for "Demonstration of repository design options". A study on "Understanding of buffering behaviour of sedimentary rock to natural perturbations" was also implemented in two areas, "evaluation of intrinsic buffering against endogenic and exogenic processes" and "development of techniques for evaluating excavation damaged zone (EDZ) self-sealing behaviour after backfilling". The Horonobe International Project (HIP) was initiated in February 2023 to promote research and development in collaboration with national and international organizations.

Development of stable solidification technique of ALPS sediment wastes by apatite ceramics (Contract research); FY2021 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Tokyo Institute of Technology*

JAEA-Review 2022-076, 227 Pages, 2023/03

JAEA-Review-2022-076.pdf:9.42MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2021. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station (1F), Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "Development of stable solidification technique of ALPS sediment wastes by apatite ceramics" conducted from FY2019 to FY2021. Since the final year of this proposal was FY2021, the results for three fiscal years were summarized. The present study aims to establish an apatite solidification process of radioactive sediment wastes, which were generated from the ALPS process manipulating the large amount of contaminated water from 1F. We selected the precipitation method and post stabilization for engineering-scale process. Investigation on composition, structure and elution properties of apatite and related phosphate waste forms fabricated from the simulated ALPS sediment wastes were implemented.

Horonobe Underground Research Laboratory Project; Investigation program for the 2022 fiscal year

Nakayama, Masashi

JAEA-Review 2022-026, 66 Pages, 2022/11

JAEA-Review-2022-026.pdf:12.31MB

The Horonobe Underground Research Laboratory (URL) Project is being pursued by the Japan Atomic Energy Agency (JAEA) to enhance the reliability of relevant disposal technologies for geological disposal of High-level Radioactive Waste through investigations of the deep geological environment within the host sedimentary rock at Horonobe Town in Hokkaido, north Japan. In fiscal year 2022, we continue to conduct research on "Study on near-field system performance in geological environment", "Demonstration of repository design options", and "Understanding of buffering behaviour of sedimentary rocks to natural perturbations", which are the important issues shown in the Horonobe underground research plan from fiscal year 2020. The main studies to be conducted in fiscal year 2022 are as follows. As "Study on near-field system performance in geological environment", we will continue to the test under the simulated condition in which the heat generation by the high-level radioactive waste has subsides in the full-scale engineered barrier system (EBS) performance experiment. We will also conduct solute transport experiment with model testing that take into account the effects of organic matter, microbes, and colloids, and initiate borehole investigation to evaluate solute transport experiments on fractures distribute in Koetoi formation. As "Demonstration of repository design concept", we will continue experiment and analysis of concrete deterioration in the underground environment as a demonstration of remote technique for emplacement and retrievable. As a demonstration of the closure techniques, laboratory tests will be continued to investigate the mechanism of bentonite runoff behaviour, which could be a factor in changing the performance of backfill material, and to expand data on swelling and deformation behaviour. In addition, in-situ borehole closure tests will be conducted to evaluate the applicability of the closure method. As "Understanding of buffering behaviour of

(Copepoda) from a deep sediment-trap; Abundance and implications for ecological and biogeochemical studies

Ikenoue, Takahito*; Otosaka, Shigeyoshi*; Honda, Makio*; Kitamura, Minoru*; Mino, Yoshihisa*; Narita, Hisashi*; Kobayashi, Takuya

Frontiers in Marine Science (Internet), 9, p.884320_1 - 884320_11, 2022/05

https://doi.org/10.3389/fmars.2022.884320

We studied seasonal variations of the mesozooplankton swimmer community collected by a sediment trap moored at 873 m in the Kuroshio & Oyashio Transition region off the east coast of Japan from 5 August 2011 to 23 June 2013. The total flux of mesozooplankton swimmers varied between 0 and 11.1 individuals m-2 d-1, with a mean of 3.1 individuals m-2 d-1 during the sampling period. Among the Copepoda, Neocalanus cristatus was the most dominant taxon. The species composition of the swimmers closely reflected the mid-depth mesozooplankton of the Oyashio region. The fluxes of Neocalanus species reflected ontogenetic vertical migration, but may have been overestimates of active fluxes if they included dormant individuals that accidentally entered the sediment trap.

Development of stable solidification technique of ALPS sediment wastes by apatite ceramics (Contract research); FY2020 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Tokyo Institute of Technology*

JAEA-Review 2021-077, 217 Pages, 2022/03

JAEA-Review-2021-077.pdf:12.34MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "Development of stable solidification technique of ALPS sediment wastes by apatite ceramics" conducted in FY2020. The present study aims to establish an apatite solidification process of radioactive sediment wastes, which were generated from the ALPS process manipulating the large amount of contaminated water from Fukushima Daiichi Nuclear Power Station. In FY2020, the synthetic scheme and elemental composition were updated to precipitation method to accept the actual ALPS sediment wastes in engineering scale. The synthesis of apatite or phosphate wastes and their molding conditions were surveyed, and the relations among elemental compositions, structures and chemical properties were clarified.

Numerical reproduction of dissolved U concentrations in a PO-treated column study of Hanford 300 area sediment using a simple ion exchange and immobile domain model

Saito, Tatsuo; Sato, Kazuhiko; Yamazawa, Hiromi*

Journal of Environmental Radioactivity, 237, p.106708_1 - 106708_9, 2021/10

https://doi.org/10.1016/j.jenvrad.2021.106708

We succeeded at numerical reproduction of dissolved U concentrations from column experiments with PO-treated Hanford 300 Area sediment. The time-series curves of dissolved U concentrations under various Darcy flow rate conditions were reproduced by the numerical model in the present study through optimization of the following parameters:(i) the mass of U in mobile domain (on surface soil connected to the stream) and the rest of the total U left as precipitation in immobile domain (isolated in deep soil);(ii) the mixing ratio between immobile and mobile domains, to fit the final recovering curve of concentration; and (iii) the cation exchange capacity (CEC) and equilibrium constant (k) of the exchange reaction of UO and H on simulated soil surface (), to fit the transient equilibrium concentration, forming the bed of the bathtub curve.

Horonobe Underground Research Laboratory Project; Investigation report for the 2019 fiscal year

Nakayama, Masashi; Saiga, Atsushi

JAEA-Review 2020-042, 116 Pages, 2021/01

JAEA-Review-2020-042.pdf:10.33MB

The Horonobe Underground Research Laboratory Project will be conducted in three phases, namely "Phase 1: Surface-based investigations", "Phase 2: Construction Phase" (investigations during construction of the underground facilities) and "Phase 3: Operation phase" (research in the underground facilities). This report summarizes the results of the investigations for the 2019 fiscal year (2019/2020). The investigations, which are composed of "Geoscientific research" and "R and D on geological disposal technology", were carried out according to "Horonobe Underground Research Laboratory Project Investigation Program for the 2019 fiscal year". The results of these investigations, along with the results which were obtained in other departments of Japan Atomic Energy Agency (JAEA), are properly offered to the implementations and the safety regulations. For the sake of this, JAEA has proceeded with the project in collaboration with experts from domestic and overseas research organizations.

Long term monitoring and evaluation of the excavation damaged zone induced around the wall of the shaft applying optical fiber sensor (Cooperative research)

Hata, Koji*; Niunoya, Sumio*; Uyama, Masao*; Nakaoka, Kenichi*; Fukaya, Masaaki*; Aoyagi, Kazuhei; Sakurai, Akitaka; Tanai, Kenji

JAEA-Research 2020-010, 142 Pages, 2020/11

JAEA-Research-2020-010.pdf:13.74MB
JAEA-Research-2020-010-appendix(DVD-ROM).zip:149.9MB

In the geological disposal study of high-level radioactive waste, it is suggested that the excavation damaged zone (EDZ) which is created around a tunnel by the excavation will be possible to be one of the critical path of radionuclides. Especially, the progress of cracks in and around the EDZ with time affects the safety assessment of geological disposal and it is important to understand the hydraulic change due to the progress of cracks in and around EDZ. In this collaborative research, monitoring tools made by Obayashi Corporation were installed at a total of 9 locations in the three boreholes near the depth of 370 m of East Shaft at the Horonobe Underground Research Laboratory constructed in the Neogene sedimentary rock. The monitoring tool consists of one set of "optical AE sensor" for measuring of the mechanical rock mass behavior and "optical pore water pressure sensor and optical temperature sensor" for measuring of groundwater behavior. This tool was made for the purpose of selecting and analyzing of AE signal waveforms due to rock fracture during and after excavation of the target deep shaft. As a result of analyzing various measurement data including AE signal waveforms, it is able to understand the information on short-term or long-term progress of cracks in and around EDZ during and after excavation in the deep shaft. In the future, it will be possible to carry out a study that contributes to the long-term stability evaluation of EDZ in sedimentary rocks in the deep part of the Horonobe Underground Research Laboratory by evaluation based on these analytical data.

Development of JAEA sorption database (JAEA-SDB); Update of sorption/QA data in FY2019

Sugiura, Yuki; Suyama, Tadahiro*; Tachi, Yukio

JAEA-Data/Code 2019-022, 40 Pages, 2020/03

JAEA-Data-Code-2019-022.pdf:2.22MB

Sorption behavior of radionuclides (RNs) in buffer materials, rocks and cementitious materials is one of the key processes in a safe geological disposal. This report focuses on updating of JAEA sorption database (JAEA-SDB) as a basis of integrated approach for the performance assessment (PA)-related distribution coefficient (K) setting and development of mechanistic sorption models. K data and their quality assurance (QA) results were updated by focusing on the following systems as potential needs extracted from our recent activities on the K setting and development of mechanistic models, i.e., clay minerals, sedimentary rocks and cementitious materials. As a result, 6,702 K data from 60 references were added and the total number of K values in JAEA-SDB reached 69,679. The QA/classified K data reached about 72% for all K data in JAEA-SDB.

The In-situ experiment for performance confirmation of engineered barrier system at Horonobe Underground Research Laboratory; Installation of engineered barrier system and backfilling the test niche at the 350m gallery

Nakayama, Masashi; Ono, Hirokazu

JAEA-Research 2019-007, 132 Pages, 2019/12

JAEA-Research-2019-007.pdf:11.29MB
JAEA-Research-2019-007-appendix(CD-ROM).zip:39.18MB

The Horonobe Underground Research Laboratory (URL) Project has being pursued by Japan Atomic Energy Agency (JAEA) to enhance the reliability of relevant disposal technologies through investigations of the deep geological environment within the host sedimentary formation at Horonobe, northern Hokkaido. The URL Project consists of two major research areas, "Geoscientific Research" and "Research and Development on Geological Disposal Technologies". The in-situ experiment for performance confirmation of engineered barrier system (EBS experiment) had been prepared from 2013 to 2014 fiscal year at GL-350m gallery, and heating by electric heater in simulated overpack had started in January, 2015. One of objectives of the EBS experiment is acquiring data concerned with Thermal-Hydrological-Mechanical-Chemical (THMC) coupled behavior. These data will be used in order to confirm the performance of engineered barrier system. This report shows following works had carried out at the GL-350 m gallery. Excavation of a test niche and a test pit, Setting buffer material blocks and a simulated overpack into the test pit, Backfilling the niche by compaction backfilling material and setting backfilling material blocks, Casting concrete type plug and contact grouting, Consolidate measurement system and start measuring.